Öйú¿ÆѧԺ´óÁ¬»¯ÎïËù³ÂÇì°²¿ÎÌâ×飨http://www.lbcs.dicp.ac.cn/£©³ÏƸ¸÷²ã´ÎÈ˲ţ¨Óлú»¯Ñ§, »¯Ñ§È˹¤ÖÇÄÜ£©
¿ÎÌâ×鳤½éÉÜ£º³ÂÇì°²£¬¸£½¨ÈªÖÝÈË¡£2007Äê±¾¿Æ±ÏÒµÓÚÖйú¿Æѧ¼¼Êõ´óѧ»¯Ñ§Ïµ£¬µ¼Ê¦ÓÈÌï°Ò½ÌÊÚ¡£2012ÄêÔÚÖйú¿ÆѧԺ´óÁ¬»¯Ñ§ÎïÀíÑо¿Ëù»ñµÃ²©Ê¿Ñ§Î»£¬µ¼Ê¦ÖÜÓÀ¹óÑо¿Ô±¡£2012ÄêÖÁ2015ÄêÔÚÃÀ¹ú¼ÓÖÝ´óѧŷÎÄ·ÖУ½øÐв©Ê¿ºóÑо¿£¬ºÏ×÷µ¼Ê¦Vy M.Dong½ÌÊÚ¡£2015ÄêÖÁ2017Äê×÷ΪµÂ¹úºé±¤Ñ§ÕßÔڵ¹ú°ØÁÖ¹¤Òµ´óѧMartin Oestreich½ÌÊÚÑо¿×鿪չ²©Ê¿ºóÑо¿¹¤×÷¡£2017Äê¼ÓÈë´óÁ¬»¯ÎïËù¿ªÕ¹¶ÀÁ¢Ñо¿¹¤×÷£¬ÈÎÑо¿×é×鳤¡£¹ú¼ÒרÏîÈ˲ÅÒý½ø¼Æ»®ÇàÄêÏîÄ¿»ñµÃÕߣ¨2017£©¡¢´óÁ¬»¯ÎïËùÕÅ´óìÏÇàÄêѧÕß¡£
×Ô¿ªÕ¹Ñо¿¹¤×÷ÒÔÀ´£¬ÒÔͨѶ×÷Õß»òµÚÒ»×÷ÕßÏȺóÔÚ¹ú¼ÊȨÍþÆÚ¿¯ÉÏ·¢±íÑо¿ÂÛÎÄ50¶àƪ£¬°üÀ¨Nature Catal.£¨1ƪ£©¡¢Nature Chem.£¨1ƪ£©¡¢Nature Commun.£¨4ƪ£©¡¢J. Am. Chem. Soc.£¨8ƪ£©¡¢Angew. Chem. Int. Ed.£¨10ƪ£©£¬Chem. Soc. Rev. (2ƪ)¡£2017Äê»ñµÃÁÉÄþÊ¡×ÔÈ»¿ÆѧһµÈ½±£¨ÅÅÃûµÚ¶þ£©¡£Ä¿Ç°Ö÷ÒªÑо¿ÁìÓòΪ·ÂÉú´ß»¯ºÏ³ÉºÍ½ðÊôÓлú»¯Ñ§¡£
¿ÎÌâ×éÖ÷ÒªÑо¿·½ÏòΪ¹ý¶É½ðÊô´ß»¯£¬ÓлúºÏ³É£¬»¯Ñ§È˹¤ÖÇÄÜ¡£ÏÖÕÐƸÑо¿Ô±¡¢¸±ÑУ¬²©Ê¿ºó£¬Ñо¿ÖúÀí£¬Ñо¿ÉúºÍÁªºÏÅàÑøÑо¿ÉúµÈ¸÷²ã´ÎÈ˲Å. ÓÐÐËȤÕßÇë·¢Ë͸öÈ˼òÀúºÍ´ú±í×÷µÈµ½£ºqachen@dicp.ac.cn, ²¢×¢Ã÷ӦƸ¸Úλ¡£¾ßÌåÒªÇóºÍ´ýÓöÈçÏ£º
£¨Ò»£©Ñо¿Ô±1Ãû£º¹¤×Ê´ýÓö¸ù¾Ý´óÁ¬»¯ÎïËùÏà¹Ø¹æ¶¨´ÓÓÅ¿¼ÂÇ£¬²¢¸ù¾Ý¹¤×÷Òµ¼¨¶îÍâ·¢·Å½òÌù¡£°´ÕÕ¹¤×Ê×ܶî×÷Ϊ»ùÊý½É´æס·¿¹«»ý½ð£¬½É´æ±ÈÀýºÏ¼Æ40%£¨µ¥Î»¸ºµ£25%£¬¸öÈË15%£©¡£
Ò»¡¢¸Úλ´ýÓö
1¡¢¾ßÓоºÕùÁ¦µÄ´ýÓö¡¢¸£ÀûµÈ£¬¾ßÌåÃæÒé¡£
2¡¢ÆäËû´ýÓö
£¨1£©×ÓÅ®¿É½øÈëÖйú¿ÆѧԺÓ׶ùÔ°¡¢´óÁ¬Àí¹¤´óѧ¸½ÊôСѧ£¨×ÛºÏÅÅÃûÈ«ÊÐÇ°Ê®£©ºÍ´óÁ¬Àí¹¤´óѧ¸½ÊôÖÐѧ£¨×ÛºÏÅÅÃûÈ«ÊÐÇ°Ê®£©¾Í¶Á£»
£¨2£©Ìṩ12¸öÔÂÃâ·ÑÈ˲Ź«Ô¢Ò»Ì×£¬Áà°üÈëס£»
£¨3£©ÐÖú½â¾öÅäż¹¤×÷£¬ÅäżÔÝʱÎÞ¹¤×÷Õߣ¬Ìṩ1500Ôª/ÔµÄÉú»î²¹Ìù£¬ÒÔ¼°×î¶à²»³¬¹ý3ÄêµÄÉç±£²¹Öú¡£
¶þ¡¢È˲ÅÕþ²ß
1¡¢¹ú¼Ò»òÖпÆÔºÈ˲żƻ®£ºÆ¸ÎªÑо¿Ô±¡¢²©µ¼£¬Ìṩ900Íò¿ÆÑÐÆô¶¯¾·ÑÖ§³Ö£¬220Íò°²¼Ò²¹Ìù¡£ÆäÖУ¬ÖпÆÔºÈ˲żƻ®¹úÄÚÍâÈ˲žù¿ÉÉêÇ룬¾ßÌåÇé¿ö¿Éµç»°×Éѯ¡£
2¡¢¡°ÕÅ´óìÏÓÅÐãѧÕß¡±£º45ÖÜËêÒÔÏ£¬ÔÚ±¾Ñ§¿ÆÁìÓòÈ¡µÃÍ»³ö³É¼¨¡¢½øÈëÊÀ½ç¿Æ¼¼Ç°ÑصÄÓÅÐãÇàÄêѧÊõ´øÍ·ÈË¡£ÌØÊâ¸Úλ½òÌù40Íò/Äִ꣬ÐÐÆÚ5Äê¡£
3¡¢¡°ÕÅ´óìÏÇàÄêѧÕß¡±£º38ÖÜËêÒÔÏ£¬ÔÚ±¾Ñ§¿ÆÁìÓòÈ¡µÃ½ÏºÃ³É¼¨¡¢ÓÐÍû½øÈëÊÀ½ç¿Æ¼¼Ç°ÑصÄÓÅÐãÇàÄê¹Ç¸ÉÈ˲š£ÌØÊâ¸Úλ½òÌù30Íò/Äִ꣬ÐÐÆÚ5Äê¡£
Èý¡¢Ó¦Æ¸ÒªÇó£º
1£©»ñµÃ²©Ê¿Ñ§Î»»ò´Óʹý²©Ê¿ºóÑо¿£¬ÔÔòÉÏÓ¦µ±µ£Èθ±¸ß¼¶×¨Òµ¼¼Êõ¼°ÒÔÉÏÖ°Îñ£»ÔÚ¿ÆѧÑо¿·½ÃæÒÑÈ¡µÃÍ»³öѧÊõ³É¹û£¬ÓнÏÇ¿µÄÍŶÓÁìµ¼ºÍ×é֯е÷ÄÜÁ¦£¬´´Ð·¢Õ¹Ç±Á¦´ó£¬¾ßÓÐÐÖú±¾Ñ§¿Æ¸Ï³¬»ò±£³Ö¹ú¼ÊÏȽøˮƽµÄÄÜÁ¦¡£
£¨¶þ£©¸±ÑÐ2Ãû£º¹¤×Ê´ýÓö¸ù¾Ý´óÁ¬»¯ÎïËùÏà¹Ø¹æ¶¨´ÓÓÅ¿¼ÂÇ£¬²¢¸ù¾Ý¹¤×÷Òµ¼¨¶îÍâ·¢·Å½òÌù¡£°´ÕÕ¹¤×Ê×ܶî×÷Ϊ»ùÊý½É´æס·¿¹«»ý½ð£¬½É´æ±ÈÀýºÏ¼Æ40%£¨µ¥Î»¸ºµ£25%£¬ ¸öÈË15%£©¡£ÁíÍâÑо¿ËùÌṩһ´ÎÐÔ20Íò°²¼Ò²¹Ìù£¬´óÁ¬ÊÐÈ˲Ű²¼Ò²¹Ìù30Íò¡£ÁíÍâÌرðÓÅÐãÕß¿ÉÒÔÐÖúÉêÇë´óÁ¬»¯ÎïËù¡°ÓÅÐãÇàÄ격ʿÈ˲š±£¬Ö±½ÓƸÓÃΪ¸±Ñо¿Ô±£¬°²¼Ò²¹Ìù50ÍòÔª£¬¿ÆÑÐÆô¶¯¾·Ñ100Íò¡£
ӦƸҪÇó£º 1£©Óлú»¯Ñ§»ò»¯Ñ§È˹¤ÖÇÄܵÈÏà¹Øרҵ²©Ê¿Ñ§Î»£¬²¢ÒÔµÚÒ»×÷ÕßÔÚJACS, AngewµÈȨÍþÆÚ¿¯·¢±íÑо¿ÂÛÎÄ£¬Óк£Íⲩºó¾ÀúÕßÓÅÏÈ¿¼ÂÇ¡£¡¡
2£©ÓÐÍŶӾ«Éñ£¬¹¤×÷̤ʵ£¬ÓÐÔðÈθУ¬Ò×¹µÍ¨ºÍÁ¼ºÃµÄÓ¢ÎÄд×÷ÄÜÁ¦¡£
3£©¼«ÆäÓÅÐãÕß¿ÉÒÔÐÖúÉêÇëÖпÆÔºÔº°ÙÈË£¨°²¼Ò²¹Ìù¹²220Íò£©£¬Ñо¿Ô±¸Ú루·Ç¶ÀÁ¢³É×飩¡£
£¨Èý£©²©Ê¿ºó2-3Ãû£¨ÓÅÐãÕß¿ÉÒÔÉêÇëÓÅÐ㲩ʿºó½±Ñ§½ð£©£º¹¤×Ê´ýÓö¸ù¾Ý´óÁ¬»¯ÎïËùÏà¹Ø¹æ¶¨´ÓÓÅ¿¼ÂÇ£¬¸ù¾Ý¹¤×÷Òµ¼¨¶îÍâ·¢·Å½òÌù£¨Ô¤¼Æ´ýÓö30-80ÍòÔª£©¡£»¯ÎïËùÓÅÐ㲩ʿºó½±Àø»ù½ð»ñµÃÕßÄêн×î¸ßÔ¼80Íò¡£³öÕ¾ºóÓÅÏÈÁôËù¹¤×÷£¬Ñо¿ËùÌṩһ´ÎÐÔ20Íò°²¼Ò²¹Ìù£¬´óÁ¬ÊÐÈ˲Ű²¼Ò²¹Ìù30Íò¡£ÌرðÓÅÐãÕßÁôËùºó¿ÉÒÔÐÖúÉêÇë´óÁ¬»¯ÎïËù¡°ÓÅÐãÇàÄ격ʿÈ˲š±£¬Ö±½ÓƸÓÃΪ¸±Ñо¿Ô±£¬°²¼Ò²¹Ìù50ÍòÔª£¬¿ÆÑÐÆô¶¯¾·Ñ100Íò¡£
ӦƸҪÇó£º 1£©½üÆÚ¼´½«»ñµÃ²©Ê¿Ñ§Î»»òÕßÒÑ»ñµÃ²©Ê¿Ñ§Î»£¬²¢ÒÔµÚÒ»×÷ÕßÔÚÓлú»¯Ñ§»ò»¯Ñ§È˹¤ÖÇÄܵÈÏà¹ØרҵÆÚ¿¯·¢±í¹ýÑо¿ÂÛÎÄ¡£2£© ²©Ê¿½×¶ÎÑо¿·½ÏòΪÓлúºÏ³É»òÕß½ðÊôÓлú»¯Ñ§£¬²¢ÓÐÁ¼ºÃµÄÓ¢ÎĿƼ¼ÂÛÎÄд×÷ÄÜÁ¦¡£3£©¹¤×÷̤ʵ£¬ÓÐÍŶӾ«Éñ£¬ÓÐÔðÈθУ¬Ò×¹µÍ¨¡£
£¨ËÄ£©ÖúÀíÑо¿Ô±£¨·ÇÃØÊé¸Ú룬2Ãû£©£º¹¤×Ê´ýÓö¸ù¾Ý´óÁ¬»¯ÎïËùÏà¹Ø¹æ¶¨´ÓÓÅ¿¼ÂÇ£¬²¢¸ù¾Ý¹¤×÷Òµ¼¨¶îÍâ·¢·Å½òÌù¡£°´ÕÕ¹¤×Ê×ܶî×÷Ϊ»ùÊý½É´æס·¿¹«»ý½ð£¬½É´æ±ÈÀýºÏ¼Æ40%£¨µ¥Î»¸ºµ£25%£¬¸öÈË15%£©¡£ÁíÍâÑо¿ËùÌṩһ´ÎÐÔ20Íò°²¼Ò²¹Ìù£¬´óÁ¬ÊÐÈ˲Ű²¼Ò²¹Ìù30Íò¡£ ÌرðÓÅÐãÕß¿ÉÒÔÐÖúÉêÇë´óÁ¬»¯ÎïËù¡°ÓÅÐãÇàÄ격ʿÈ˲š±£¬Ö±½ÓƸÓÃΪ¸±Ñо¿Ô±£¬°²¼Ò²¹Ìù50ÍòÔª£¬¿ÆÑÐÆô¶¯¾·Ñ100Íò¡£
ӦƸҪÇó£º 1£©½üÆÚ¼´½«»ñµÃ²©Ê¿Ñ§Î»»òÕßÒÑ»ñµÃ²©Ê¿Ñ§Î»£¬Óлú»¯Ñ§»ò»¯Ñ§È˹¤ÖÇÄܵÈÏà¹Øרҵ¡£2£©Ó¢ÓïÁ¼ºÃ£¬ÄܶÀÁ¢ÔĶÁÓ¢ÎÄÎÄÏײ¢¿ªÕ¹Ñо¿¿ÎÌ⣬²¢ÒÔµÚÒ»×÷ÕßÔÚÓлú»¯Ñ§×¨ÒµÆÚ¿¯·¢±í¹ýÑо¿ÂÛÎÄ¡£3£©ÊìϤ³£¹æ»¯Ñ§ÊµÑé¼¼ÊõºÍ²Ù×÷¹¤×÷̤ʵ£¬ÓÐÔðÈθУ¬¾ßÓÐÁ¼ºÃµÄ¹µÍ¨ÄÜÁ¦ºÍºÏ×÷¾«Éñ¡£
ÓÐÐËȤÕßÇë·¢Ë͸öÈ˼òÀúºÍ´ú±í×÷µÈµ½£ºqachen@dicp.ac.cn, ²¢×¢Ã÷ӦƸ¸Úλ¡£
´ú±íÐÔÂÛÎÄ£¨½ü4Ä꣬ͨѶ×÷Õߣ©
[1] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2023, 62, e202317299.
[2] Yuan, W.* Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2023, 62, e202314304.
[3] Chen, Q. A.* et al. Nature Commun. 2023, 14, 7087.
[4] Ji, D. W.* Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2023, 62, e202300036.
[5] Chen, Q. A.* et al. Nature Commun. 2023, 14, 651.
[6] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2023, 62, e202213074.
[7] Chen, Q. A.* et al. Nature Catal. 2022, 5, 708.
[8] Zheng, J.;* Chen, Q. A.;* Ma, S.* et al. Nature Chem. 2022, 14, 1185.
[9] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2022, 61, e202207202.
[10] Chen, Q. A.* et al. J. Am. Chem. Soc. 2022, 144, 11081.
[11] Chen, Q. A.* et al. Nature Commun. 2022, 13, 3496.
[12] Chen, Q. A.* et al. Nature Commun. 2021, 12, 6538.
[13] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2021, 60, 24284.
[14] Jiang, X. L.;* Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2021, 60, 8321.
[15] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2021, 60, 1583.
[16] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2020, 59, 19115.
[17] Chen, Q. A.* et al. Angew. Chem. Int. Ed. 2019, 58, 5438. |